Found as a drop by the Sorebones, Skull staples are used by Dr. Fenkenstrain in The Great Brain Robbery quest along with a pair of brain tongs, bell jars and a cranial clamp. This equipment is used to perform brain transplants on the zombified monks in Mos Le'Harmless in order to restore them to their normal form. Strangely, if a group of skull staples are examined, the examine text will still be 'One skull staple'.
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